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Paper titanyl sensor sees H2O2 vapor at 0.04 ppb

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Ammonium titanyl oxalate on cellulose turns yellow as a Ti(IV)–peroxide complex, detecting hydrogen peroxide vapor down to about 0.04 ppb without fancy instrumentation.

Source

Designing Tunable Paper-Based Colorimetric Sensor for Precise Detection of Hydrogen Peroxide Vapor

Hossain R, Apblett A, Materer NF · ACS omega · 2025

doi.org/10.1021/acsomega.5c01380Read the full paper ↗0 citationscc by

Study at a glance

Design
Other — Ammonium titanyl oxalate paper sensor calibrated against H2O2 vapor
N
Analytical sensing method — no sample cohort N
Population
Paper-based colorimetric sensors exposed to H2O2 vapor
Outcome
Colorimetric LOD and selectivity for hydrogen peroxide vapor (~0.04 ppb)

Structured fields used in claim comparison tables when every cited study has a complete layer.

What they did

Authors drop-cast ammonium titanyl oxalate on paper towels, characterised Ti–peroxo formation by UV–vis, FTIR and XPS, and calibrated color/absorbance versus H2O2 vapor generated from diluted 30 wt% solutions.

What they found

Colorless-to-yellow change peaking near 400 nm; LOD ≈ 0.04 ppb from 0.0025 AU noise and 0.187 AU ppb−1 sensitivity; first-order vapor-diffusion kinetics; high selectivity versus water, O2 and common solvents.

The limits

What it doesn't show

Field deployment against real IED plumes or long-term humidity cycling is not demonstrated—calibration used sealed-container vapors above aqueous H2O2.

Key terms

Titanyl oxalate
Ammonium titanyl oxalate, a Ti(IV) precursor that binds peroxide.
Ti(IV)–peroxide complex
Coordination complex that absorbs near 400 nm and appears bright yellow.
LOD
Limit of detection, here ~0.04 ppb H2O2 vapor.
Colorimetric sensor
Device that reports analyte concentration by a visible color change.
Cellulose microfibrils
Porous paper fibers providing high surface area for the titanyl salt.

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The yellow color comes from:

Common questions

What color change is observed?

Colorless to bright yellow, λmax ≈ 400 nm.

What LOD is reported?

0.04 ppb.

How is the paper prepared?

Drop-cast 100 μL titanyl solution on 2.5×2.5 cm paper, vacuum dry 1 h.

What XPS O 1s feature indicates peroxide?

A secondary peak near 535 eV assigned to O–O.

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