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Nonlinear optics

Can light-matter hybrids broaden a laser pulse on a tiny chip?

Walker PM, Whittaker CE, Skryabin DV, et al. · Light, science & applications · 2019

Open access · cc by · source: Europe PMC

Mixing light with semiconductor excitons made a short laser pulse spread into a broad rainbow of colours and angles using far less power and length than ordinary optical materials need.

Study at a glance

Design
Other — Picosecond laser pulses coupled into a GaAs quantum-well polariton waveguide at 10 K; output spectra recorded versus wavelength and angle, compared with numerical solutions of coupled photon-exciton equations.
N
No sample size; one waveguide device measured at several powers, detunings and propagation lengths.
Population
A planar GaAs-based waveguide strongly coupled to quantum-well excitons
Outcome
Spectral and angular broadening of output pulses and the mechanisms producing it

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Key findings

At low power the spectrum broadened by self-phase modulation, more strongly on the side closer to the exciton because those polaritons are more matter-like and more nonlinear; simulations reproduced the spectra and predicted the pulse splitting into a train of roughly 450 fs pulses. At intermediate and high powers, extra emission followed curves predicted by spatiotemporal modulation instability and by Cherenkov/X-wave phase matching. The total spectrum widened up to 30 meV, about 11 times the input width, with peak coupled powers of at most 110 W.

Methodology

The team sent 2-picosecond laser pulses into a gallium arsenide waveguide cooled to 10 K, where light couples strongly to excitons to form polaritons. They measured the output light as a function of wavelength and transverse angle while varying pulse power, device length and how far the laser frequency sat from the exciton resonance. They compared the low-power spectra with numerical solutions of coupled photon and exciton equations, and the high-power patterns with analytic predictions for modulation instability and Cherenkov emission.

Limitations

The sub-picosecond pulse splitting and curved wavefronts come from simulations, because the experiment could not measure such fast time dynamics directly. The device works at 10 K and in GaAs, where the light-matter coupling strength caps the achievable broadening, so room-temperature operation in other materials is only proposed. Short-wavelength emission was absorbed by the exciton tail, hiding part of the predicted spectrum, and the high-power regime involves several mixed processes that are hard to separate cleanly.

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