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Persistent pollutants

Serum PFAS mixes reveal seafood vs product exposure

Hu XC, Dassuncao C, Zhang X, et al. · Environmental health : a global access science source · 2018

Open access · cc by · source: Europe PMC

Long-chain PFCAs mark seafood/whale diets, while PFHxS and N-EtFOSAA mark carpets and consumer products in children.

Key findings

Whalers’ profiles were ~80% PFOS and separated on PC1 (51% of variance). Children had higher PFHxS and N-EtFOSAA. Hair mercury correlated with PFHpS, PFDA, PFOS, and PFUnDA (ρ 0.35–0.61). Carpets raised PFHxS 37.2% in NHANES. Seafood tracked PFNA in both US cohorts.

Methodology

Authors compared 15 PFASs in Faroese children, women, and whalers, ran PCA/clustering, and modeled NHANES 2005–06 and CHirP predictors such as seafood, carpets, and drinking water.

Limitations

NHANES models explained only 9–25% of PFAS variance. Toxicokinetics and time trends can mimic source differences. CHirP detected only four PFASs in >50% of people.

How this study connects

Role on claims

Each row is a claim on a concept or method page where this paper supports, challenges, or qualifies the statement. Roles are hand-checked — not a model guess.

  • SupportsPersistent pollutantsconcept

    Long-chain PFCAs mark seafood/whale diets, while PFHxS and N-EtFOSAA mark carpets and consumer products in children.

    Evidence for the claim as stated.

  • SupportsBiomonitoringmethod

    PFAS profiles can separate sources but explain little variance. Faroese whalers' mixes were ~80% PFOS and separated on PC1 (51% of variance); children's profiles were richer in PFHxS and N-EtFOSAA. Hair mercury correlated with PFHpS, PFDA, PFOS and PFUnDA (ρ 0.35–0.61). In NHANES, carpets raised PFHxS 37.2% and seafood tracked PFNA, yet the models explained only 9–25% of PFAS variance.

    Evidence for the claim as stated.

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